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She essayed the role of a film star opposite Ram Kapoor, Evelyn Sharma and Navdeep Chabbra.The film emerged to be a critical and commercial failure.and shared that she keeps her body in shape by working out as much as she can despite her busy schedule and as quoted in Men's Fitness magazine, "I try to eat very healthy – lots of vegetables, drinking my milk every day." In 2013, Leone posed for a PETA ad campaign, encouraging dog and cat owners to have their pets spayed and neutered.In an interview for PETA India, Leone said, "I believe that every single dog should be spayed and neutered.She was named Penthouse Pet of the Year in 2003, was a contract performer for Vivid Entertainment, and was named by Maxim as one of the 12 top porn stars in 2010.She has played roles in independent mainstream events, films and television shows.She indicated that for the right price she would seriously consider a career in Bollywood.In 2008, Leone announced that she would be starring in a mainstream action adventure movie titled Pirates Blood, which was shot in Oman.
The film released to mixed reviews and was an average earner.The movie led to her being nominated for three (out of six) AVN awards in 2009 in addition to being a choice for Female Performer of the Year.She followed up her first boy-girl title with The Other Side of Sunny in October 2008, which would be the last time she would perform with Erikson. She indicated in an April 2012 interview that 80 per cent of the traffic on her website, and 60 per cent of her revenue comes from India.In January 2008, Leone revealed that she was no longer exclusive to Erikson, and had done scenes with other actors, most notably Tommy Gunn, Charles Dera, James Deen Her websites and business interests are run under her banner company Leone L. In 2013, she announced her retirement from the adult industry stating "I am lucky that the audience is accepting me. I don't have any plans as of now to go back there." A police first information report was filed against her in May 2015 after a woman at Mumbai, India, complained that Leone's website, sunnyleone.com, was destroying the Indian culture.Thane police's cyber cell at Ramnagar booked her for sections 292, 292A, 294 which could land her into jail, fine or both.
In May 2007, upon re-signing her contract with Vivid for another six films, Leone agreed to perform for the first time with men on camera, but exclusively with her fiancé, Matt Erikson.